Volume 2 Issue 4
December  2023
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Wanyao Zhang, Yufang Chen, Hongjing Gao, Wei Xie, Peng Gao, Chunman Zheng, Peitao Xiao. Review of regulating Zn2+ solvation structures in aqueous zinc-ion batteries[J]. Materials Futures, 2023, 2(4): 042102. doi: 10.1088/2752-5724/ace3de
Citation: Wanyao Zhang, Yufang Chen, Hongjing Gao, Wei Xie, Peng Gao, Chunman Zheng, Peitao Xiao. Review of regulating Zn2+ solvation structures in aqueous zinc-ion batteries[J]. Materials Futures, 2023, 2(4): 042102. doi: 10.1088/2752-5724/ace3de
shu
Topical Review •
OPEN ACCESS

Review of regulating Zn2+ solvation structures in aqueous zinc-ion batteries

© 2023 The Author(s). Published by IOP Publishing Ltd on behalf of the Songshan Lake Materials Laboratory
Materials Futures, Volume 2, Number 4
  • Received Date: 2023-06-07
  • Accepted Date: 2023-07-04
  • Revised Date: 2023-07-01
  • Publish Date: 2023-08-04
doi: 10.1088/2752-5724/ace3de
  • 1.

    College of Aerospace Science and Engineering, National University of Defense Technology, Changsha, Hunan 410073, People’s Republic of China

  • 2.

    College of Materials Science and Engineering, Hunan Joint International Laboratory of Advanced Materials and Technology of Clean Energy, Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology, Hunan University, Changsha 410082, People’s Republic of China

  • Author’s contribution

    P Xiao conducted Project administration, writing-original draft, writing-review & editing, funding acquisition, and conceptualization. W Zhang conducted writing-original draft. Y Chen and C Zheng conducted supervision. H Gao, P Gao, and W Xie conducted validation and writing-review & editing.

    W Z and P X contribute equally to this work.

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    Abstract
  • Aqueous zinc-ion batteries, due to their high power density, intrinsic safety, low cost, and environmental benign, have attracted tremendous attentions recently. However, their application is severely plagued by the inferior energy density and short cycling life, which was mainly ascribed to zinc dendrites, and interfacial side reactions, narrow potential window induced by water decomposition, all of which are highly related with the Zn2+ solvation structures in the aqueous electrolytes. Therefore, in this review, we comprehensively summarized the recent development of strategies of regulating Zn2+ solvation structures, specially, the effect of zinc salts, nonaqueous co-solvents, and functional additives on the Zn2+ solvation structures and the corresponding electrochemical performance of aqueous zinc-ion batteries. Moreover, future perspectives focused on the challenges and possible solutions for design and commercialization of aqueous electrolytes with unique solvation structures are provided.
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    • Conflict of interest

    There are no conflicts to declare.

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