Volume 1 Issue 2
June  2022
Turn off MathJax
Article Contents
Qiang Luo, Zichao Wei, Hanyi Duan, Lei Jin, Rumasha N T Kankanamage, Seth Shuster, Steven L Suib, James F Rusling, Jie He. Templated synthesis of crystalline mesoporous CeO2 with organosilane-containing polymers: balancing porosity, crystallinity and catalytic activity[J]. Materials Futures, 2022, 1(2): 025302. doi: 10.1088/2752-5724/ac7605
Citation: Qiang Luo, Zichao Wei, Hanyi Duan, Lei Jin, Rumasha N T Kankanamage, Seth Shuster, Steven L Suib, James F Rusling, Jie He. Templated synthesis of crystalline mesoporous CeO2 with organosilane-containing polymers: balancing porosity, crystallinity and catalytic activity[J]. Materials Futures, 2022, 1(2): 025302. doi: 10.1088/2752-5724/ac7605
Paper •
OPEN ACCESS

Templated synthesis of crystalline mesoporous CeO2 with organosilane-containing polymers: balancing porosity, crystallinity and catalytic activity

© 2022 The Author(s). Published by IOP Publishing Ltd on behalf of the Songshan Lake Materials Laboratory
Materials Futures, Volume 1, Number 2
  • Received Date: 2022-04-26
  • Accepted Date: 2022-06-05
  • Rev Recd Date: 2022-06-01
  • Publish Date: 2022-06-22
  • We report the synthesis of ordered mesoporous ceria (mCeO2) with highly crystallinity and thermal stability using hybrid polymer templates consisting of organosilanes. Those organosilane-containing polymers can convert into silica-like nanostructures that further serve as thermally stable and mechanically strong templates to prevent the collapse of mesoporous frameworks during thermal-induced crystallization. Using a simple evaporation-induced self-assembly process, control of the interaction between templates and metal precursors allows the co-self-assembly of polymer micelles and Ce3+ ions to form uniform porous structures. The porosity is well-retained after calcination up to 900 C. After the thermal engineering at 700 C for 12 h (mCeO2-700-12 h), mCeO2 still has a specific surface area of 96 m2 g-1 with a pore size of 14 nm. mCeO2 is demonstrated to be active for electrochemical oxidation of sulfite. mCeO2-700-12 h with a perfect balance of crystallinity and porosity shows the fastest intrinsic activity that is about 84 times more active than bulk CeO2 and 5 times more active than mCeO2 that has a lower crystallinity.
  • loading
  • [1]
    Taguchi A, Schth F 2005 Microporous Mesoporous Mater. 77 1-45 doi: 10.1016/j.micromeso.2004.06.030
    [2]
    Rao Y, Antonelli D M 2009 J. Mater. Chem. 19 1937-44 doi: 10.1039/b813533a
    [3]
    Kuo C-H, et al 2015 ACS Catal. 5 1693-9 doi: 10.1021/cs501739e
    [4]
    Lu X, Ng Y H, Zhao C 2014 ChemSusChem 7 82-6 doi: 10.1002/cssc.201300975
    [5]
    Luo W, Li Y, Dong J, Wei J, Xu J, Deng Y, Zhao D 2013 Angew. Chem., Int. Ed. 52 10505-10 doi: 10.1002/anie.201303353
    [6]
    Zu L, Zhang W, Qu L, Liu L, Li W, Yu A, Zhao D 2020 Adv. Energy Mater. 10 2002152 doi: 10.1002/aenm.202002152
    [7]
    Xiong H, Zhou H, Sun G, Liu Z, Zhang L, Zhang L, Du F, Qiao Z A, Dai S 2020 Angew. Chem., Int. Ed. 59 11053-60 doi: 10.1002/anie.202002051
    [8]
    Brezesinski T, Wang J, Tolbert S H, Dunn B 2010 Nat. Mater. 9 146-51 doi: 10.1038/nmat2612
    [9]
    Xu F, Jin S, Zhong H, Wu D, Yang X, Chen X, Wei H, Fu R, Jiang D 2015 Sci. Rep. 5 1-6 doi: 10.1038/srep08225
    [10]
    Joo J B, Dahl M, Li N, Zaera F, Yin Y 2013 Energy Environ. Sci. 6 2082-92 doi: 10.1039/c3ee41155a
    [11]
    Tanaka M, Shima H, Yokoi T, Tatsumi T, Kondo J N 2011 Catal. Lett. 141 283-92 doi: 10.1007/s10562-010-0458-1
    [12]
    Ismail A A, Bahnemann D W 2011 J. Mater. Chem. 21 11686-707 doi: 10.1039/c1jm10407a
    [13]
    Ismail A A, Bahnemann D W, Robben L, Yarovyi V, Wark M 2010 Chem. Mater. 22 108-16 doi: 10.1021/cm902500e
    [14]
    Onozuka K, Kawakami Y, Imai H, Yokoi T, Tatsumi T, Kondo J 2012 J. Solid State Chem. 192 87-92 doi: 10.1016/j.jssc.2012.03.055
    [15]
    Hurum D C, Agrios A G, Gray K A, Rajh T, Thurnauer M C 2003 J. Phys. Chem. B 107 4545-9 doi: 10.1021/jp0273934
    [16]
    Kawahara T, Konishi Y, Tada H, Tohge N, Nishii J, Ito S 2002 Angew. Chem., Int. Ed. 41 2811-3 doi: 10.1002/1521-3773(20020802)41:15<2811::AID-ANIE2811>3.0.CO;2;2-%23
    [17]
    Zhang L, Jin L, Liu B, He J 2019 Front. Chem. 7 22 doi: 10.3389/fchem.2019.00022
    [18]
    Yue W, Zhou W 2008 Prog. Nat. Sci. 18 1329-38 doi: 10.1016/j.pnsc.2008.05.010
    [19]
    Kondo J N, Domen K 2008 Chem. Mater. 20 835-47 doi: 10.1021/cm702176m
    [20]
    Liu F, Liu C-L, Hu B, Kong W-P, Qi C-Z 2012 Appl. Surf. Sci. 258 7448-54 doi: 10.1016/j.apsusc.2012.04.059
    [21]
    Zhang Z, Zuo F, Feng P 2010 J. Mater. Chem. 20 2206-12 doi: 10.1039/b921157h
    [22]
    Cop P, Kitano S, Niinuma K, Smarsly B, Kozuka H 2018 Nanoscale 10 7002-15 doi: 10.1039/C8NR00793D
    [23]
    Zhang X, Yu X, Zhou B, Luo W, Jiang W, Jiang W, Shen Z, Wang L 2015 J. Am. Ceram. Soc. 98 1056-9 doi: 10.1111/jace.13529
    [24]
    Liang C, Li Z, Dai S 2008 Angew. Chem., Int. Ed. 47 3696-717 doi: 10.1002/anie.200702046
    [25]
    Liu B, et al 2015 Angew. Chem., Int. Ed. 54 9061-5 doi: 10.1002/anie.201502892
    [26]
    Lu A H, Schth F 2006 Adv. Mater. 18 1793-805 doi: 10.1002/adma.200600148
    [27]
    Jiao F, Bruce P G 2007 Adv. Mater. 19 657-60 doi: 10.1002/adma.200602499
    [28]
    Deng X, Chen K, Tysz H 2017 Chem. Mater. 29 40-52 doi: 10.1021/acs.chemmater.6b02645
    [29]
    Cho H S, Ryoo R 2012 Microporous Mesoporous Mater. 151 107-12 doi: 10.1016/j.micromeso.2011.11.007
    [30]
    Kruk M, Dufour B, Celer E B, Kowalewski T, Jaroniec M, Matyjaszewski K 2005 J. Phys. Chem. B 109 9216-25 doi: 10.1021/jp045594x
    [31]
    Jin L, Liu B, Wu Y, Thanneeru S, He J 2017 ACS Appl. Mater. Interfaces 9 36837-48 doi: 10.1021/acsami.7b11453
    [32]
    Malgras V, AtaeeEsfahani H, Wang H, Jiang B, Li C, Wu K C W, Kim J H, Yamauchi Y 2016 Adv. Mater. 28 993-1010 doi: 10.1002/adma.201502593
    [33]
    Wang H, Jeong H Y, Imura M, Wang L, Radhakrishnan L, Fujita N, Castle T, Terasaki O, Yamauchi Y 2011 J. Am. Chem. Soc. 133 14526-9 doi: 10.1021/ja2058617
    [34]
    Li W, Zhao D 2013 Chem. Commun. 49 943-6 doi: 10.1039/C2CC36964H
    [35]
    Ren Y, Ma Z, Bruce P G 2012 Chem. Soc. Rev. 41 4909-27 doi: 10.1039/c2cs35086f
    [36]
    Gu D, Schth F 2014 Chem. Soc. Rev. 43 313-44 doi: 10.1039/c3cs60155b
    [37]
    Yang P, Zhao D, Margolese D I, Chmelka B F, Stucky G D 1998 Nature 396 152-5 doi: 10.1038/24132
    [38]
    Yun H S, Miyazawa K C, Zhou H, Honma I, Kuwabara M 2001 Adv. Mater. 13 1377-80 doi: 10.1002/1521-4095(200109)13:18<1377::AID-ADMA1377>3.0.CO;2-T
    [39]
    Lee J, Christopher Orilall M, Warren S C, Kamperman M, Disalvo F J, Wiesner U 2008 Nat. Mater. 7 222-8 doi: 10.1038/nmat2111
    [40]
    Zhang R, Tu B, Zhao D 2010 Chem. Eur. J. 16 9977-81 doi: 10.1002/chem.201001241
    [41]
    Wan Y, Zhao D 2007 Chem. Rev. 107 2821-60 doi: 10.1021/cr068020s
    [42]
    Poyraz A S, Kuo C-H, Biswas S, King’ondu C K, Suib S L 2013 Nat. Commun. 4 2952 doi: 10.1038/ncomms3952
    [43]
    Li W, et al 2011 Adv. Energy Mater. 1 382-6 doi: 10.1002/aenm.201000096
    [44]
    Jin L, et al 2020 Adv. Funct. Mater. 30 1909491 doi: 10.1002/adfm.201909491
    [45]
    Jin L, Liu B, Louis M E, Li G, He J 2020 ACS Appl. Mater. Interfaces 12 9617-27 doi: 10.1021/acsami.9b20231
    [46]
    Hu M, Jin L, Su X, Bamonte S, Lu X, Gao P, Suib S L, Liu B, He J 2020 ChemCatChem 12 1476-82 doi: 10.1002/cctc.201901957
    [47]
    Hu M, Jin L, Dang Y, Suib S L, He J, Liu B 2020 Front. Chem. 8 581512 doi: 10.3389/fchem.2020.581512
    [48]
    Liu B, Jin L, Zheng H, Yao H, Wu Y, Lopes A, He J 2017 ACS Appl. Mater. Interfaces 9 1746-58 doi: 10.1021/acsami.6b11958
    [49]
    Liu B, Yao H, Daniels R A, Song W, Zheng H, Jin L, Suib S L, He J 2016 Nanoscale 8 5441-5 doi: 10.1039/C6NR00604C
    [50]
    Liu B, Luo Z, Federico A, Song W, Suib S L, He J 2015 Chem. Mater. 27 6173-6 doi: 10.1021/acs.chemmater.5b02248
    [51]
    Li W, Kuo C-H, Kanyo I, Thanneeru S, He J 2014 Macromolecules 47 5932-41 doi: 10.1021/ma501338s
    [52]
    Du J, Chen Y 2005 Macromol. Rapid Commun. 26 491-4 doi: 10.1002/marc.200400579
    [53]
    Montini T, Melchionna M, Monai M, Fornasiero P 2016 Chem. Rev. 116 5987-6041 doi: 10.1021/acs.chemrev.5b00603
    [54]
    Dav-Quionero A, Navlani-Garca M, Lozano-Castello D, Bueno-Lpez A, Anderson J A 2016 ACS Catal. 6 1723-31 doi: 10.1021/acscatal.5b02741
    [55]
    Vinodkumar T, Rao B G, Reddy B M 2015 Catal. Today 253 57-64 doi: 10.1016/j.cattod.2015.01.044
    [56]
    Mullins D, Zhang K 2002 Surf. Sci. 513 163-73 doi: 10.1016/S0039-6028(02)01704-1
    [57]
    Durgasri D N, Vinodkumar T, Lin F, Alxneit I, Reddy B M 2014 Appl. Surf. Sci. 314 592-8 doi: 10.1016/j.apsusc.2014.07.036
    [58]
    Li S, et al 2017 Angew. Chem., Int. Ed. 56 10761-5 doi: 10.1002/anie.201705002
    [59]
    Ji P, Zhang J, Chen F, Anpo M 2008 J. Phys. Chem. C 112 17809-13 doi: 10.1021/jp8054087
    [60]
    Roggenbuck J, Schfer H, Tsoncheva T, Minchev C, Hanss J, Tiemann M 2007 Microporous Mesoporous Mater. 101 335-41 doi: 10.1016/j.micromeso.2006.11.029
    [61]
    Laha S, Ryoo R 2003 Chem. Commun. 17 2138-9 doi: 10.1039/B305524H
    [62]
    Vickers S M, Gholami R, Smith K J, MacLachlan M J 2015 ACS Appl. Mater. Interfaces 7 11460-6 doi: 10.1021/acsami.5b02367
    [63]
    Kresge A C, Leonowicz M, Roth W J, Vartuli J, Beck J 1992 Nature 359 710-2 doi: 10.1038/359710a0
    [64]
    Pan J H, Zhao X, Lee W I 2011 Chem. Eng. J. 170 363-80 doi: 10.1016/j.cej.2010.11.040
    [65]
    Bass J D, Grosso D, Boissiere C, Sanchez C 2008 J. Am. Chem. Soc. 130 7882-97 doi: 10.1021/ja078140x
    [66]
    Crepaldi E L, Soler-Illia G J D A, Grosso D, Cagnol F, Ribot F, Sanchez C 2003 J. Am. Chem. Soc. 125 9770-86 doi: 10.1021/ja030070g
    [67]
    Ansari S A, Khan M M, Ansari M O, Kalathil S, Lee J, Cho M H 2014 RSC Adv. 4 16782-91 doi: 10.1039/C4RA00861H
    [68]
    Zhang J, et al 2011 Adv. Energy Mater. 1 241-8 doi: 10.1002/aenm.201000004
    [69]
    Mahoney L, Koodali R T 2014 Materials 7 2697-746 doi: 10.3390/ma7042697
    [70]
    Amri F, Septiani N L W, Rezki M, Iqbal M, Yamauchi Y, Golberg D, Kaneti Y V, Yuliarto B 2021 J. Mater. Chem. B 9 1189-207 doi: 10.1039/D0TB02292F
    [71]
    Dahal N, Ibarra I A, Humphrey S M 2012 J. Mater. Chem. 22 12675-81 doi: 10.1039/c2jm30460k
    [72]
    Wang J, Li H, Li H, Zou C, Wang H, Li D 2014 ACS Appl. Mater. Interfaces 6 1623-31 doi: 10.1021/am404484k
    [73]
    Fan X, Wang T, Guo Y, Gong H, Xue H, Guo H, Gao B, He J 2017 Microporous Mesoporous Mater. 240 1-8 doi: 10.1016/j.micromeso.2016.10.049
    [74]
    Hao C, Lv H, Mi C, Song Y, Ma J 2016 ACS Sustain. Chem. Eng. 4 746-56 doi: 10.1021/acssuschemeng.5b00531
    [75]
    Jin L, Liu C-H, Cintron D, Luo Q, Nieh M-P, He J 2021 Langmuir 37 9865-72 doi: 10.1021/acs.langmuir.1c01554
    [76]
    Kraffert K, Karg M, Schmack R, Clavel G, Boissiere C, Wirth T, Pinna N, Kraehnert R 2018 Adv. Mater. Interfaces 5 1800360 doi: 10.1002/admi.201800360
    [77]
    Schilling C, Hofmann A, Hess C, Ganduglia-Pirovano M V 2017 J. Phys. Chem. C 121 20834-49 doi: 10.1021/acs.jpcc.7b06643
    [78]
    Silva I D C, Sigoli F A, Mazali I O 2017 J. Phys. Chem. C 121 12928-35 doi: 10.1021/acs.jpcc.7b03155
    [79]
    Guhel Y, Ta M, Bernard J, Boudart B, Pesant J 2009 J. Raman Spectrosc. 40 401-4 doi: 10.1002/jrs.2140
    [80]
    O’brien J, Hinkley J, Donne S, Lindquist S-E 2010 Electrochim. Acta 55 573-91 doi: 10.1016/j.electacta.2009.09.067
    [81]
    Zelinsky A, Pirogov B Y 2017 Electrochim. Acta 231 371-8 doi: 10.1016/j.electacta.2017.02.070
    [82]
    Kim T W, Choi K-S 2014 Science 343 990-4 doi: 10.1126/science.1246913
    [83]
    Randviir E P 2018 Electrochim. Acta 286 179-86 doi: 10.1016/j.electacta.2018.08.021
    [84]
    Sharma A, Bhattarai J K, Nigudkar S S, Pistorio S G, Demchenko A V, Stine K J 2016 J. Electroanal. Chem. 782 174-81 doi: 10.1016/j.jelechem.2016.10.013
  • 加载中

Catalog

    Figures(8)  / Tables(1)

    Article Metrics

    Article Views(466) PDF downloads(74)
    Article Statistics
    Related articles from

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return