Volume 2 Issue 4
December  2023
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Wanyao Zhang, Yufang Chen, Hongjing Gao, Wei Xie, Peng Gao, Chunman Zheng, Peitao Xiao. Review of regulating Zn2+ solvation structures in aqueous zinc-ion batteries[J]. Materials Futures, 2023, 2(4): 042102. doi: 10.1088/2752-5724/ace3de
Citation: Wanyao Zhang, Yufang Chen, Hongjing Gao, Wei Xie, Peng Gao, Chunman Zheng, Peitao Xiao. Review of regulating Zn2+ solvation structures in aqueous zinc-ion batteries[J]. Materials Futures, 2023, 2(4): 042102. doi: 10.1088/2752-5724/ace3de
shu
Topical Review •
OPEN ACCESS

Review of regulating Zn2+ solvation structures in aqueous zinc-ion batteries

© 2023 The Author(s). Published by IOP Publishing Ltd on behalf of the Songshan Lake Materials Laboratory
Materials Futures, Volume 2, Number 4
  • Received Date: 2023-06-07
  • Accepted Date: 2023-07-04
  • Publish Date: 2023-08-04
doi: 10.1088/2752-5724/ace3de

  • 1 College of Aerospace Science and Engineering, National University of Defense Technology, Changsha, Hunan 410073, People’s Republic of China

  • 2 College of Materials Science and Engineering, Hunan Joint International Laboratory of Advanced Materials and Technology of Clean Energy, Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology, Hunan University, Changsha 410082, People’s Republic of China

Funds:

This work was supported by Natural Science Foundation of Hunan Province (2023JJ40662), National Defense Science and Technology Key Laboratory Supporting Project (WDZC20235250508), National Natural Science Foundation (22002186), Seed Fund of National University of Defense Technology.

    Abstract
  • Aqueous zinc-ion batteries, due to their high power density, intrinsic safety, low cost, and environmental benign, have attracted tremendous attentions recently. However, their application is severely plagued by the inferior energy density and short cycling life, which was mainly ascribed to zinc dendrites, and interfacial side reactions, narrow potential window induced by water decomposition, all of which are highly related with the Zn2+ solvation structures in the aqueous electrolytes. Therefore, in this review, we comprehensively summarized the recent development of strategies of regulating Zn2+ solvation structures, specially, the effect of zinc salts, nonaqueous co-solvents, and functional additives on the Zn2+ solvation structures and the corresponding electrochemical performance of aqueous zinc-ion batteries. Moreover, future perspectives focused on the challenges and possible solutions for design and commercialization of aqueous electrolytes with unique solvation structures are provided.
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